One, I've actually been in the room where the lasers pump a trial accelerator similar to what is in that linked cartoon.
That said, get rid of the static by classical means. The pulsed laser you need for air breakdown over a tiny path costs 55,000$ and up just for the laser. That's not counting the means you need to have to sweep the beam back and forth etc. You cannot do it with a continuous wave laser, and it is hugely impractical to do it with a pulsed laser. Reason being is the practical laser can only zap a cubic millimeter at most at one time. If you have really specialized optics, you might ionize a two cm long thin thread at best. That's not going to help you clear a calendaring roll in a machine. Even if you scan the beam, you'd hit repetition rate issues with available lasers.
Conductive materials, Antistatic Materials , changes in calendaring roller tribology, humidifiers, neutralized ion sources, pre-spaying an opposite charge, atmospheric pressure plasma machines etc ...
ALL of them work far, far far, far, far better then a laser induced breakdown for this task.
I do photonics for a living. One of my concerns used to be air breakdown on the faces of glass optics and non-linear crystals. I've sat and watched a tiny plasma ball form on my dead skin more then once. I know the mechanism quite well. This is not a cost effective means to use a nanosecond, picosecond, or femtosecond pulsed laser.
This is state of the art, made using several graduate students, probably upwards of 100,000 USD worth of technology, and several man-years of work.
https://youtu.be/AoWi10YVmfEIt clearly would not cover a high speed calendaring roll.
Steve