I've managed to charge them up decently with a Buck converter and a high power 24V DC power supply but the buck converter is limited in terms of power and needs around 5 minutes to fully charge.
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What would be the best way to charge them up quickly?
I suggest a bigger buck converter. Or several in parallel. You might be able to come up with one that has
input current limiting which will make maximum use of your 24V supply.
Also, Ogden is dead right about needing some balancing between caps.
By my calculations you have some 30kJ or more on hand. That’s a
lot, so be careful! Eye protection is a must, because you don’t want hot chunks of metal in your eyes. Ear protection is probably advisable as well. And gloves to protect you from hot chunks of that-
used-to-be-my-good-spanner.
Finally, remember to fit some discharge resistors so that this bank will eventually reach 0V on its own (rather than wait for weeks and surprise you).