The ground pour looks reasonable, but with a switching converter the critical issue is loop area, not simply having plenty of ground copper. Keep the input ceramic capacitor directly between VIN and the IC ground/PowerPAD, and make the high-current loop through the IC, catch diode and input capacitor as short and wide as possible.
Also:
Keep the SW copper small and away from FB, COMP and RT/CLK traces.
Take the feedback divider’s ground from the quiet output-capacitor ground, not from the diode’s noisy return path.
Connect the exposed PowerPAD firmly to ground with several thermal vias.
Keep the output capacitor close to the inductor and diode return.
Decide consistently whether mounting holes are grounded; chassis mounting holes should not be connected accidentally.
I would compare the placement and routing directly against TI’s
TPS54560 datasheet example layout and
evaluation-module layout. Those are better references than judging the ground pour alone.