Last ISE (14.7) supports the 3 family and is still available. If it weren't, it would mean that then 6 series would also be "dead", as ISE is the only way of dealing with it. Which is far from being true.
As woofy said, I would also suggest switching to a newer family for new designs, but I suspect ISE will still be usable in many years from now. If you're on Windows 10, though, you will need to use a virtual machine - I think Xilinx provides a ready-to-use install for Windows 10 using a VM. Or, you can use ISE on Linux.