GLCD is a peripheral for controlling segment LCD displays. SAM C2x don't have that, only SAM L2x devices have that peripheral. But it is also useless for ST7789.
There is not support for ST7789 in Harmony, so you would have to either make a driver yourself or use one of many available from various sources. It will not fit exactly into the Harmony ecosystem, so you would just have to use SPI or whatever interface your display supports and bridge that to the actual driver.
If you want to use graphical library from Harmony, then your only option is to implement the driver in a way that meets the requirements of the graphics library. There is a generic driver that can be used as a template, but I don't think it will work as is.
The only demo application for the SAM C20/C21 (gfx_apps_sam_c20_c21/tree/master/apps/legato_quickstart) uses ILI9488 driver, which should be close to ST7789 in principle. But it is not something you can just drag and drop, some manual programming would be required.
Also, keep in mind that ST7789 does not support 5V operation, so you need to make sure you use appropriate level shifters.