Okay with that new asc file I can get it to run.
May be not. Take a look in the image. Only I keep open the CLK pin. Did you check test_UC3825.asc waveform, it seems same.
But again its shows this error, \UC3825N\UC3825_based_pwm_control_ps.net(26): File not found.
.lib ..\sym\ValVol\ValVol.lib
^^^^^^^^^^^^^^^^^^^^^^^^
Okay I think I see your problem. Those ValVol symbols contain a reference to the relative path
..\sym\ValVol\ValVol.lib. The person who created this library/symbols must have set this up, but on your machine this path likely does not exist. But LTspice is still looking for it, hence the error message.
So what you want to do is remove the reference to that path from the symbol file.
1. Open the symbol file in LTspice.
2. Go to Edit > Attributes > Edit Attributes.
3. In the SpiceModel field you'll see the path "..\sym\ValVol\ValVol.lib". Delete this.
4. Close the Symbol Attribute Editor Window. Save the symbol.
5. Go back to the schematic view. Delete the UC3825 symbol from the schematic.
6. Open the component browser and find the UC3825 symbol. Cick "Refresh" (if you don't do this first, the changes to the symbol might not apply).
7. Add the symbol to the schematic again.
8. It should run fine, assuming you have a proper .inc statement for ValVol.lib in the schematic.
Alternatively, for step 3 can replace the path with just "ValVol.lib". If you do this then you don't need the .inc statement in the schematic.