Fast answer: The motor limits your max RPM
The pololu can supply up to 2A with a heatsink and air flow (1A without heatsink). Your stepper motor has rated current 0.6A.
Take care not to burn the pololu or your stepper motor. When you set the output current treat the potentiometer gently. Trust me on that, I've got at least 5 stepsticks burned when I calibrated my reprap. One full rotation has a HUGE impact on the output current. Try 45° steps or smaller when you turn the potentiometer.
The limits of a stepper motor that are usually declared on the motor specifications document.
http://sine.ni.com/ds/app/doc/p/id/ds-311/lang/en , search for "Max Speed rpm"
In your case, the max speed is not declared but you can calculate it.
You can find some on-line calculators. I hope this one
http://www.daycounter.com/Calculators/Stepper-Motor-Calculator.phtml works for you.
The stepper does not rotate with constant speed. During each step, the motor shaft accelerates for a part of the step and it decelerates until it reaches the next step position where it's rotational speed goes back to zero (actually it fluctuates a bit near the ideal position because the controller continuously makes tiny corrections , especially when you use microstepping).
The stepper motor has a maximum torque limit.
The torque needed to overcome the inertia of the moving parts limits your maximum RPM.
http://en.wikipedia.org/wiki/Angular_acceleration