I think a little less than one third, I only removed some on the top. The dag cable is connected to some wipe contacts on the bottom of the crt and this part is intact with the original aquadag.
Also could that be related to the amount of static charge/discharge noise when the screen is turned on or off because I think it increased
From reading a bit on the internet I think it would normally discharge through the aquadag but if there is less of it it will also discharge through the air and cause more of this noise and a bit of a shock if you touch the screen and ground when turning it off
"a little less than one third" falls nicely into my 'not sure' range! If you'd said 50% I'd say too much, if you'd said 25% I'd say it's fine. So it's a bit less than a third then it's
probably fine.

It sounds as if the grounding of the remaining aquadag is nicely intact - you'd see internal sparks to the spring or hear a loud crack otherwise. I think the reason for a little more static sound at turn on and off could possibly be because the lower capacitance allows the EHT to rise and drop faster, the same with the increased static feel on the screen (you always get a fair amount anyway). It could just as easily be that you have now 'fixated' on it because of what you did, whereas before, you simply weren't listening or conscious of it. You don't normally go feeling for static day-to-day. To me, CRT TVs always seemed to make a bit more static sound after a good cleaning anyway.
The real test of insufficient EHT capacitance is sudden picture size changes when scenes change on the program, especially going from a dark to light scene - there is always a little but if it is now excessive and distracting then you probably need to do something.
I would go for James's suggestion of carbon paint if you really do need to do anything. Aquadag is a fairly high resistance coating anyway. Thinking overnight, Aluminium tape might be a bad idea - if it eventually curled up with the heat and fell down into the electronics, you would have real problems! Otherwise, I'd leave it alone, it won't cause any damage to the circuit.