It will be hard to calibrate such a device - you need radioactive material with known spectrum for calibration. In university we had used Americium and Strontium, but such a materials are under control of agencies for nuclear safety. If you will be able to get it, than you will have lot of fun with photomultiplier tube used for the signal amplification. I have doubts that someone can get something more modern for "home" use. In case that you can measure energy of each pulse, than with calibration you can find what you are looking at (from the histogram of detected energies).
IT-65 is able to catch decay from lead (it is always slightly radioactive due to the isotope which is in nature), so it can be somehow useful, in case the intensity is too high than the shutter in the front of detector tube should can be closed. When is something slightly radioactive it starts "ticking". What you need is counter tube with widow like mentioned Philips tube, which is able to detect Alpha particles. I suspect that eastern block was not able to produce such a tubes and thus they were imported from west. Commonly available Geiger counter tubes on ebay are useless. They are made from metal and the sensitivity is poor even for bigger ones.